Transition from simple to complex behavior of single molecule line shapes in disordered condensed phase

E. Barkai; R. Silbey; G. Zumofen

doi:10.1063/1.1288905

Transition from simple to complex behavior of single molecule line shapes in disordered condensed phase

E. Barkai, R. Silbey, G. Zumofen

Research output: Contribution to journal › Article › peer-review

25 Scopus citations

Abstract

The spectral line shapes of single molecules (SMs) embedded in a randomly distributed two levels system (TLS) have been investigated using the Kubo-Anderson sudden jump approach. The SMs exhibited a wide variety of behaviors in the random environment. The behaviors were analyzed using tunneling and glass models.

Original language	English
Pages (from-to)	5853-5867
Number of pages	15
Journal	Journal of Chemical Physics
Volume	113
Issue number	14
DOIs	https://doi.org/10.1063/1.1288905
State	Published - 8 Oct 2000
Externally published	Yes

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abstract = "The spectral line shapes of single molecules (SMs) embedded in a randomly distributed two levels system (TLS) have been investigated using the Kubo-Anderson sudden jump approach. The SMs exhibited a wide variety of behaviors in the random environment. The behaviors were analyzed using tunneling and glass models.",

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Transition from simple to complex behavior of single molecule line shapes in disordered condensed phase

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