Time-dependent fluctuations in single molecule spectroscopy: A generalized wiener-khintchine approach

Eli Barkai; Youn Joon Jung; Robert Silbey

doi:10.1103/physrevlett.87.207403

Time-dependent fluctuations in single molecule spectroscopy: A generalized wiener-khintchine approach

Eli Barkai
, Youn Joon Jung
, Robert Silbey

Massachusetts Institute of Technology

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

We consider the theory of time-dependent fluctuations in single molecule spectroscopy. In particular, the relation between stationary spectral diffusion processes and photon counting statistics is investigated. Within linear response theory, a general relation between Mandel’s Q parameter and a three time dipole correlation function is obtained. For a prototype spectral diffusion process, an exact solution of Q is found which exhibits rich types of physical behaviors.

Original language	English
Pages (from-to)	207403-1-207403-4
Journal	Physical Review Letters
Volume	87
Issue number	20
DOIs	https://doi.org/10.1103/physrevlett.87.207403
State	Published - 12 Nov 2001
Externally published	Yes

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10.1103/physrevlett.87.207403

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abstract = "We consider the theory of time-dependent fluctuations in single molecule spectroscopy. In particular, the relation between stationary spectral diffusion processes and photon counting statistics is investigated. Within linear response theory, a general relation between Mandel{\textquoteright}s Q parameter and a three time dipole correlation function is obtained. For a prototype spectral diffusion process, an exact solution of Q is found which exhibits rich types of physical behaviors.",

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AB - We consider the theory of time-dependent fluctuations in single molecule spectroscopy. In particular, the relation between stationary spectral diffusion processes and photon counting statistics is investigated. Within linear response theory, a general relation between Mandel’s Q parameter and a three time dipole correlation function is obtained. For a prototype spectral diffusion process, an exact solution of Q is found which exhibits rich types of physical behaviors.

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Time-dependent fluctuations in single molecule spectroscopy: A generalized wiener-khintchine approach

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