Time-dependent fluctuations in single molecule spectroscopy: A generalized wiener-khintchine approach

E. Barkai, Y. J. Jung, R. Silbey

Research output: Contribution to journalArticlepeer-review

81 Scopus citations

Abstract

The important time ordering properties of a three time correlation function C3τ12τ3 are evaluated as well as Mandel's Q parameter. It is shown that the relation between the function and line shape fluctuations described by Q generalizes the Wiener-Khintchine theorem, that relates the averaged line shape and the one time dipole correlation function.

Original languageEnglish
Article number207403
Pages (from-to)207403/1-207403/4
JournalPhysical Review Letters
Volume87
Issue number20
StatePublished - 12 Nov 2001
Externally publishedYes

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