The origin of anomalous temperature dependences of intensities of spin-forbidden d-d transitions in octahedral complexes

A. V. Malakhovskii, G. G. Vasiljev

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Abstract

It is shown that anomalous temperature dependences of intensities of spin-forbidden d-d transitions, observed in octahedral magnetically-ordering complexes in a paramagnetic phase and in particular in hexagonal RbMnCl3, investigated by the authors, can be accounted for by a pair-vibrational mechanism, which represents two simultaneous events: breaking of selection rules for spin during pair absorption by exchange coupled ions and breaking of those for parity during an ordinary electronic transition in one of the ions of the pair due to excitation of odd-parity vibrations.

Original languageEnglish
Pages (from-to)353-356
Number of pages4
JournalSolid State Communications
Volume48
Issue number4
DOIs
StatePublished - Oct 1983
Externally publishedYes

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