The Magnetic Genome of Two-Dimensional van der Waals Materials

Qing Hua Wang; Amilcar Bedoya-Pinto; Mark Blei; Avalon H. Dismukes; Assaf Hamo; Sarah Jenkins; Maciej Koperski; Yu Liu; Qi Chao Sun; Evan J. Telford; Hyun Ho Kim; Mathias Augustin; Uri Vool; Jia Xin Yin; Lu Hua Li; Alexey Falin; Cory R. Dean; Fèlix Casanova; Richard F.L. Evans; Mairbek Chshiev; Artem Mishchenko; Cedomir Petrovic; Rui He; Liuyan Zhao; Adam W. Tsen; Brian D. Gerardot; Mauro Brotons-Gisbert; Zurab Guguchia; Xavier Roy; Sefaattin Tongay; Ziwei Wang; M. Zahid Hasan; Joerg Wrachtrup; Amir Yacoby; Albert Fert; Stuart Parkin; Kostya S. Novoselov; Pengcheng Dai; Luis Balicas; Elton J.G. Santos

doi:10.1021/acsnano.1c09150

The Magnetic Genome of Two-Dimensional van der Waals Materials

Qing Hua Wang, Amilcar Bedoya-Pinto, Mark Blei, Avalon H. Dismukes, Assaf Hamo, Sarah Jenkins, Maciej Koperski, Yu Liu, Qi Chao Sun, Evan J. Telford, Hyun Ho Kim, Mathias Augustin, Uri Vool, Jia Xin Yin, Lu Hua Li, Alexey Falin, Cory R. Dean, Fèlix Casanova, Richard F.L. Evans, Mairbek ChshievArtem Mishchenko, Cedomir Petrovic, Rui He, Liuyan Zhao, Adam W. Tsen, Brian D. Gerardot, Mauro Brotons-Gisbert, Zurab Guguchia, Xavier Roy, Sefaattin Tongay, Ziwei Wang, M. Zahid Hasan, Joerg Wrachtrup, Amir Yacoby, Albert Fert, Stuart Parkin, Kostya S. Novoselov, Pengcheng Dai, Luis Balicas, Elton J.G. Santos

Research output: Contribution to journal › Review article › peer-review

193 Scopus citations

Abstract

Magnetism in two-dimensional (2D) van der Waals (vdW) materials has recently emerged as one of the most promising areas in condensed matter research, with many exciting emerging properties and significant potential for applications ranging from topological magnonics to low-power spintronics, quantum computing, and optical communications. In the brief time after their discovery, 2D magnets have blossomed into a rich area for investigation, where fundamental concepts in magnetism are challenged by the behavior of spins that can develop at the single layer limit. However, much effort is still needed in multiple fronts before 2D magnets can be routinely used for practical implementations. In this comprehensive review, prominent authors with expertise in complementary fields of 2D magnetism (i.e., synthesis, device engineering, magneto-optics, imaging, transport, mechanics, spin excitations, and theory and simulations) have joined together to provide a genome of current knowledge and a guideline for future developments in 2D magnetic materials research.

Original language	English
Journal	ACS Nano
DOIs	https://doi.org/10.1021/acsnano.1c09150
State	Published - 20 Apr 2022
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2022 The Authors. Published by American Chemical Society.

Funding

X.R., C.R.D., E.J.T., and A.H.D. acknowledge support from the Center for Precision Assembly of Superstratic and Superatomic Solids, a U.S. National Science Foundation (NSF) MRSEC (award nos. DMR-2011738 and DMR-1420634), the Air Force Office of Scientific Research (award no. FA9550-18-1-0020), and the Center on Programmable Quantum Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under award DE-SC0019443. H.H.K. acknowledges funding by the National Research Foundation of Korea Grant funded by the Korean Government (NRF-2021R1C1C1012394). This project was supported by the Ministry of Education (Singapore) through the Research Centre of Excellence program (grant EDUN C-33-18-279-V12, I-FIM). B.D.G., supported by a Wolfson Merit Award from the Royal Society and a Chair in Emerging Technology from the Royal Academy of Engineering, acknowledges the EPSRC (grant no. EP/P029892/1), the ERC (grant no. 725920), the EU Horizon 2020 research and innovation program under grant agreement no. 820423. M.B.-G. is supported by a University Research Fellowship from the Royal Society (ref URF/R1/211484). L.Z. acknowledges support by NSF CAREER grant no. DMR-174774 and AFOSR grant no. FA9550- 21-1-0065. J.W. acknowledges EU project ASTERIQS and European Research Council via SMeL DFG GRK 2642 and FOR 2724. A.Y. acknowledges support from the Army Research Office (ARO) through grant no. W911NF-17-1-0023, the Quantum Science Center (QSC), a National Quantum Information Science Research Center of the U.S. Department of Energy (DOE), the Gordon and Betty Moore Foundation through grant GBMF 9468, and the STC Center for Integrated Quantum Materials, NSF grant no. DMR-1231319. Y.L., L.B., and C.P. thank Milorad Milosevic for useful communication. Work at Brookhaven National Laboratory is supported by the Office of Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy (DOE) under contract no. DE-SC0012704. L.B. is supported by the US-DOE through the BES program, award DE-SC0002613. The National High Magnetic Field Laboratory acknowledges support from the US-NSF Cooperative agreement Grant number DMR-1644779 and the state of Florida. The μSR experiments were carried out at the Swiss Muon Source (SμS) of the Paul Scherrer Institute using low background GPS (πM3 beamline) and high pressure GPD (μE1 beamline) instruments. The μSR time spectra were analysed using the free software package MUSRFIT. Z.G. gratefully acknowledges the financial support by the Swiss National Science Foundation (SNF fellowships P2ZHP2-161980 and P300P2-177832). A.F., F.C., and M.C. acknowledge European Union Horizon 2020 research and innovation programme under grant agreement no. 881603 (Graphene Flagship), Spanish MICINN under the Maria de Maeztu Units of Excellence Programme (no. MDM-2016–0618) and under project no. RTI2018-094861-B-100, French ANR MAGICVALLEY (ANR-18-CE24-0007) and discussions with P. Seneor, B. Dlubak, V. Cros, N. Reyren, H. X. Yang, A. Hallal, F. Ibrahim, F. Bonell, and M. Jamet. S.T. and M.B. acknowledge support from NSF DMR-1904716, NSF DMR-2111812, NSF ECCS-2052527, and DOE-SC0020653. The work on van der Waals materials at Rice University was supported by NSF DMR-1700081, DMR-2100741, and by the Robert A. Welch Foundation under grant no. C-1839 (P. D.). A.M. and Z.W. acknowledge the support of the EPSRC Early Career Fellowship (EP/N007131/1), the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (grant agreement no. 865590), and the Royal Society International Exchanges 2019 Cost Share Program (IEC/R2/192001). S.J. acknowledges funding by the German Research Foundation (DFG) project no. 320163632 (EV 196/2). This project made use of of the viking cluster, a high performance computing facility provided by the University of York. R.F.L.E. gratefully acknowledges the financial support of ARCHER UK National Supercomputing Service via the embedded CSE programme (ecse1307). Q.H.W. acknowledges support from NSF grants QLCI-CG-1936882 and DMR-1906030. E.J.G.S. acknowledges computational resources through CIRRUS Tier-2 HPC Service (ec131 Cirrus Project) at EPCC ( http://www.cirrus.ac.uk ) funded by the University of Edinburgh and EPSRC (EP/P020267/1); ARCHER UK National Supercomputing Service ( http://www.archer.ac.uk ) via Project d429. EJGS acknowledges the Spanish Ministry of Science’s grant program “Europa-Excelencia” under grant number EUR2020-112238, the EPSRC Early Career Fellowship (EP/T021578/1), and the University of Edinburgh for funding support. A.B.-P. acknowledges support by the Generalitat Valenciana (CIDEGENT/2021/005).

Funders	Funder number
ANR-18-CE24-0007	DMR-1700081, DMR-2111812, DMR-1904716, DOE-SC0020653, DMR-2100741, ECCS-2052527
EU Horizon 2020 research and innovation program	DMR-174774, 820423, URF/R1/211484
National Quantum Information Science Research Center
Quantum Science Center
STC Center for Integrated Quantum Materials	DMR-1231319
US-DOE	DE-SC0002613
US-NSF	DMR-1644779
National Science Foundation
U.S. Department of Energy
Air Force Office of Scientific Research	FA9550- 21-1-0065, FA9550-18-1-0020
Army Research Office	W911NF-17-1-0023
Welch Foundation	C-1839, EP/N007131/1
Gordon and Betty Moore Foundation	GBMF 9468
Office of Science
Basic Energy Sciences	DE-SC0019443
Horizon 2020 Framework Programme	865590, IEC/R2/192001, 725920
Division of Materials Sciences and Engineering	DE-SC0012704
Materials Research Science and Engineering Center, Harvard University	DMR-1420634, DMR-2011738
Engineering and Physical Sciences Research Council	EP/P029892/1
Royal Academy of Engineering
Royal Society
European Commission	DFG GRK 2642, FOR 2724
University of Edinburgh	EP/P020267/1
Deutsche Forschungsgemeinschaft	DMR-1906030, EV 196/2, QLCI-CG-1936882, ecse1307, 320163632
Agence Nationale de la Recherche
Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung	P2ZHP2-161980, P300P2-177832
Generalitat Valenciana	CIDEGENT/2021/005
National Research Foundation of Korea	NRF-2021R1C1C1012394
Ministerio de Ciencia e Innovación	EUR2020-112238, EP/T021578/1, RTI2018-094861-B-100, MDM-2016–0618
Horizon 2020	881603
Kementerian Pendidikan Malaysia	EDUN C-33-18-279-V12

Keywords

2D magnetic materials
CrI
FeGeTe
atomistic spin dynamics
magnetic genome
magneto-optical effect
neutron scattering
van der Waals

Access to Document

10.1021/acsnano.1c09150

Cite this

Wang, Q. H., Bedoya-Pinto, A., Blei, M., Dismukes, A. H., Hamo, A., Jenkins, S., Koperski, M., Liu, Y., Sun, Q. C., Telford, E. J., Kim, H. H., Augustin, M., Vool, U., Yin, J. X., Li, L. H., Falin, A., Dean, C. R., Casanova, F., Evans, R. F. L., ... Santos, E. J. G. (2022). The Magnetic Genome of Two-Dimensional van der Waals Materials. ACS Nano. https://doi.org/10.1021/acsnano.1c09150

@article{67eeb8c6601d4598ab6dad6827d824ad,

title = "The Magnetic Genome of Two-Dimensional van der Waals Materials",

abstract = "Magnetism in two-dimensional (2D) van der Waals (vdW) materials has recently emerged as one of the most promising areas in condensed matter research, with many exciting emerging properties and significant potential for applications ranging from topological magnonics to low-power spintronics, quantum computing, and optical communications. In the brief time after their discovery, 2D magnets have blossomed into a rich area for investigation, where fundamental concepts in magnetism are challenged by the behavior of spins that can develop at the single layer limit. However, much effort is still needed in multiple fronts before 2D magnets can be routinely used for practical implementations. In this comprehensive review, prominent authors with expertise in complementary fields of 2D magnetism (i.e., synthesis, device engineering, magneto-optics, imaging, transport, mechanics, spin excitations, and theory and simulations) have joined together to provide a genome of current knowledge and a guideline for future developments in 2D magnetic materials research.",

keywords = "2D magnetic materials, CrI, FeGeTe, atomistic spin dynamics, magnetic genome, magneto-optical effect, neutron scattering, van der Waals",

author = "Wang, {Qing Hua} and Amilcar Bedoya-Pinto and Mark Blei and Dismukes, {Avalon H.} and Assaf Hamo and Sarah Jenkins and Maciej Koperski and Yu Liu and Sun, {Qi Chao} and Telford, {Evan J.} and Kim, {Hyun Ho} and Mathias Augustin and Uri Vool and Yin, {Jia Xin} and Li, {Lu Hua} and Alexey Falin and Dean, {Cory R.} and F{\`e}lix Casanova and Evans, {Richard F.L.} and Mairbek Chshiev and Artem Mishchenko and Cedomir Petrovic and Rui He and Liuyan Zhao and Tsen, {Adam W.} and Gerardot, {Brian D.} and Mauro Brotons-Gisbert and Zurab Guguchia and Xavier Roy and Sefaattin Tongay and Ziwei Wang and Hasan, {M. Zahid} and Joerg Wrachtrup and Amir Yacoby and Albert Fert and Stuart Parkin and Novoselov, {Kostya S.} and Pengcheng Dai and Luis Balicas and Santos, {Elton J.G.}",

note = "Publisher Copyright: {\textcopyright} 2022 The Authors. Published by American Chemical Society.",

year = "2022",

month = apr,

day = "20",

doi = "10.1021/acsnano.1c09150",

language = "אנגלית",

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Wang, QH, Bedoya-Pinto, A, Blei, M, Dismukes, AH, Hamo, A, Jenkins, S, Koperski, M, Liu, Y, Sun, QC, Telford, EJ, Kim, HH, Augustin, M, Vool, U, Yin, JX, Li, LH, Falin, A, Dean, CR, Casanova, F, Evans, RFL, Chshiev, M, Mishchenko, A, Petrovic, C, He, R, Zhao, L, Tsen, AW, Gerardot, BD, Brotons-Gisbert, M, Guguchia, Z, Roy, X, Tongay, S, Wang, Z, Hasan, MZ, Wrachtrup, J, Yacoby, A, Fert, A, Parkin, S, Novoselov, KS, Dai, P, Balicas, L & Santos, EJG 2022, 'The Magnetic Genome of Two-Dimensional van der Waals Materials', ACS Nano. https://doi.org/10.1021/acsnano.1c09150

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AU - Bedoya-Pinto, Amilcar

AU - Blei, Mark

AU - Dismukes, Avalon H.

AU - Hamo, Assaf

AU - Jenkins, Sarah

AU - Koperski, Maciej

AU - Liu, Yu

AU - Sun, Qi Chao

AU - Telford, Evan J.

AU - Kim, Hyun Ho

AU - Augustin, Mathias

AU - Vool, Uri

AU - Yin, Jia Xin

AU - Li, Lu Hua

AU - Falin, Alexey

AU - Dean, Cory R.

AU - Casanova, Fèlix

AU - Evans, Richard F.L.

AU - Chshiev, Mairbek

AU - Mishchenko, Artem

AU - Petrovic, Cedomir

AU - He, Rui

AU - Zhao, Liuyan

AU - Tsen, Adam W.

AU - Gerardot, Brian D.

AU - Brotons-Gisbert, Mauro

AU - Guguchia, Zurab

AU - Roy, Xavier

AU - Tongay, Sefaattin

AU - Wang, Ziwei

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AU - Yacoby, Amir

AU - Fert, Albert

AU - Parkin, Stuart

AU - Novoselov, Kostya S.

AU - Dai, Pengcheng

AU - Balicas, Luis

AU - Santos, Elton J.G.

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N2 - Magnetism in two-dimensional (2D) van der Waals (vdW) materials has recently emerged as one of the most promising areas in condensed matter research, with many exciting emerging properties and significant potential for applications ranging from topological magnonics to low-power spintronics, quantum computing, and optical communications. In the brief time after their discovery, 2D magnets have blossomed into a rich area for investigation, where fundamental concepts in magnetism are challenged by the behavior of spins that can develop at the single layer limit. However, much effort is still needed in multiple fronts before 2D magnets can be routinely used for practical implementations. In this comprehensive review, prominent authors with expertise in complementary fields of 2D magnetism (i.e., synthesis, device engineering, magneto-optics, imaging, transport, mechanics, spin excitations, and theory and simulations) have joined together to provide a genome of current knowledge and a guideline for future developments in 2D magnetic materials research.

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The Magnetic Genome of Two-Dimensional van der Waals Materials

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