Temperature-dependence of the chirality-induced spin selectivity effect—Experiments and theory

Seif Alwan, Subhajit Sarkar, Amos Sharoni, Yonatan Dubi

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

The temperature-dependence of the chirality-induced spin selectivity (CISS) effect can be used to discriminate between different theoretical proposals for the mechanism of the CISS effect. Here, we briefly review key experimental results and discuss the effect of temperature in different models for the CISS effect. We then focus on the recently suggested spinterface mechanism and describe the different possible effects temperature can have within this model. Finally, we analyze in detail recent experimental results presented in the work of Qian et al. [Nature 606, 902-908 (2022)] and demonstrate that, contrary to the original interpretation by the authors, these data actually indicate that the CISS effect increases with decreasing temperature. Finally, we show how the spinterface model can accurately reproduce these experimental results.

Original languageEnglish
Article number014106
JournalJournal of Chemical Physics
Volume159
Issue number1
DOIs
StatePublished - 7 Jul 2023

Bibliographical note

Publisher Copyright:
© 2023 Author(s).

Fingerprint

Dive into the research topics of 'Temperature-dependence of the chirality-induced spin selectivity effect—Experiments and theory'. Together they form a unique fingerprint.

Cite this