Quantum dot-dye bilayer-sensitized solar cells: Breaking the limits imposed by the low absorbance of dye monolayers

Menny Shalom, Josep Albero, Zion Tachan, Eugenia Martínez-Ferrero, Arie Zaban, Emilio Palomares

Research output: Contribution to journalArticlepeer-review

136 Scopus citations

Abstract

Here, we present a new DSSC design, consisting of sequential QDs and dye sensitization layers, that opens the path toward high optical density DSSCs that cover a significant part of the solar spectrum. The new configuration is enabled by the application of an amorphous TiO2 layer between the two sensitizers, allowing both electron injection from the outer absorber and fast hole extraction from the inner sensitizing layer. Utilizing two sensitizing layers, we obtain a 250% increase in cell efficiency compared to a QD monolayer cell.

Original languageEnglish
Pages (from-to)1134-1138
Number of pages5
JournalJournal of Physical Chemistry Letters
Volume1
Issue number7
DOIs
StatePublished - 1 Apr 2010

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