Microscopic structure of the wetting film at the surface of liquid ga-bi alloys

H. Tostmann, E. Di Masi, O. G. Shpyrko, P. S. Pershan, B. M. Ocko, M. Deutsch

Research output: Contribution to journalArticlepeer-review

62 Scopus citations

Abstract

X-ray reflectivity measurements of the binary liquid Ga-Bi alloy reveal a dramatically different surface structure above and below the monotectic temperature mono = 222°C. A Gibbs-adsorbed Bi monolayer resides at the surface in both regimes. However, a 30 Å thick, Bi-rich wetting film intrudes between the Bi monolayer and the Ga-rich bulk for T > Tmono. The wetting film's internal structure, not hitherto measured, is determined with Å resolution, showing a concentration gradient not predicted by theory and a highly diffuse interface with the bulk phase.

Original languageEnglish
Pages (from-to)4385-4388
Number of pages4
JournalPhysical Review Letters
Volume84
Issue number19
DOIs
StatePublished - 2000

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