Magnesium- and intermetallic alloys-based hydrides for energy storage: Modelling, synthesis and properties

Luca Pasquini; Kouji Sakaki; Etsuo Akiba; Mark D. Allendorf; Ebert Alvares; Josè R. Ares; Dotan Babai; Marcello Baricco; Josè Bellosta Von Colbe; Matvey Bereznitsky; Craig E. Buckley; Young Whan Cho; Fermin Cuevas; Patricia De Rango; Erika Michela Dematteis; Roman V. Denys; Martin Dornheim; J. F. Fernández; Arif Hariyadi; Bjørn C. Hauback; Tae Wook Heo; Michael Hirscher; Terry D. Humphries; Jacques Huot; Isaac Jacob; Torben R. Jensen; Paul Jerabek; Shin Young Kang; Nathan Keilbart; Hyunjeong Kim; Michel Latroche; F. Leardini; Haiwen Li; Sanliang Ling; Mykhaylo V. Lototskyy; Ryan Mullen; Shin Ichi Orimo; Mark Paskevicius; Claudio Pistidda; Marek Polanski; Julián Puszkiel; Eugen Rabkin; Martin Sahlberg; Sabrina Sartori; Archa Santhosh; Toyoto Sato; Roni Z. Shneck; Magnus H. Sørby; Yuanyuan Shang; Vitalie Stavila; Jin Yoo Suh; Suwarno Suwarno; Le Thi Thu; Liwen F. Wan; Colin J. Webb; Matthew Witman; Chubin Wan; Brandon C. Wood; Volodymyr A. Yartys

doi:10.1088/2516-1083/ac7190

Magnesium- and intermetallic alloys-based hydrides for energy storage: Modelling, synthesis and properties

Luca Pasquini, Kouji Sakaki, Etsuo Akiba, Mark D. Allendorf, Ebert Alvares, Josè R. Ares, Dotan Babai, Marcello Baricco, Josè Bellosta Von Colbe, Matvey Bereznitsky, Craig E. Buckley, Young Whan Cho, Fermin Cuevas, Patricia De Rango, Erika Michela Dematteis, Roman V. Denys, Martin Dornheim, J. F. Fernández, Arif Hariyadi, Bjørn C. HaubackTae Wook Heo, Michael Hirscher, Terry D. Humphries, Jacques Huot, Isaac Jacob, Torben R. Jensen, Paul Jerabek, Shin Young Kang, Nathan Keilbart, Hyunjeong Kim, Michel Latroche, F. Leardini, Haiwen Li, Sanliang Ling, Mykhaylo V. Lototskyy, Ryan Mullen, Shin Ichi Orimo, Mark Paskevicius, Claudio Pistidda, Marek Polanski, Julián Puszkiel, Eugen Rabkin, Martin Sahlberg, Sabrina Sartori, Archa Santhosh, Toyoto Sato, Roni Z. Shneck, Magnus H. Sørby, Yuanyuan Shang, Vitalie Stavila, Jin Yoo Suh, Suwarno Suwarno, Le Thi Thu, Liwen F. Wan, Colin J. Webb, Matthew Witman, Chubin Wan, Brandon C. Wood, Volodymyr A. Yartys

Research output: Contribution to journal › Review article › peer-review

55 Scopus citations

Abstract

Hydrides based on magnesium and intermetallic compounds provide a viable solution to the challenge of energy storage from renewable sources, thanks to their ability to absorb and desorb hydrogen in a reversible way with a proper tuning of pressure and temperature conditions. Therefore, they are expected to play an important role in the clean energy transition and in the deployment of hydrogen as an efficient energy vector. This review, by experts of Task 40 'Energy Storage and Conversion based on Hydrogen' of the Hydrogen Technology Collaboration Programme of the International Energy Agency, reports on the latest activities of the working group 'Magnesium- and Intermetallic alloys-based Hydrides for Energy Storage'. The following topics are covered by the review: multiscale modelling of hydrides and hydrogen sorption mechanisms; synthesis and processing techniques; catalysts for hydrogen sorption in Mg; Mg-based nanostructures and new compounds; hydrides based on intermetallic TiFe alloys, high entropy alloys, Laves phases, and Pd-containing alloys. Finally, an outlook is presented on current worldwide investments and future research directions for hydrogen-based energy storage.

Original language	English
Article number	032007
Journal	Progress in Energy
Volume	4
Issue number	3
DOIs	https://doi.org/10.1088/2516-1083/ac7190
State	Published - 1 Jul 2022
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2022 The Author(s). Published by IOP Publishing Ltd.

Keywords

catalysts
energy storage
hydrogen storage materials
intermetallic alloys
magnesium
multiscale modelling
nanostructure

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1088/2516-1083/ac7190

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Pasquini, L., Sakaki, K., Akiba, E., Allendorf, M. D., Alvares, E., Ares, J. R., Babai, D., Baricco, M., Bellosta Von Colbe, J., Bereznitsky, M., Buckley, C. E., Cho, Y. W., Cuevas, F., De Rango, P., Dematteis, E. M., Denys, R. V., Dornheim, M., Fernández, J. F., Hariyadi, A., ... Yartys, V. A. (2022). Magnesium- and intermetallic alloys-based hydrides for energy storage: Modelling, synthesis and properties. Progress in Energy, 4(3), Article 032007. https://doi.org/10.1088/2516-1083/ac7190

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title = "Magnesium- and intermetallic alloys-based hydrides for energy storage: Modelling, synthesis and properties",

abstract = "Hydrides based on magnesium and intermetallic compounds provide a viable solution to the challenge of energy storage from renewable sources, thanks to their ability to absorb and desorb hydrogen in a reversible way with a proper tuning of pressure and temperature conditions. Therefore, they are expected to play an important role in the clean energy transition and in the deployment of hydrogen as an efficient energy vector. This review, by experts of Task 40 'Energy Storage and Conversion based on Hydrogen' of the Hydrogen Technology Collaboration Programme of the International Energy Agency, reports on the latest activities of the working group 'Magnesium- and Intermetallic alloys-based Hydrides for Energy Storage'. The following topics are covered by the review: multiscale modelling of hydrides and hydrogen sorption mechanisms; synthesis and processing techniques; catalysts for hydrogen sorption in Mg; Mg-based nanostructures and new compounds; hydrides based on intermetallic TiFe alloys, high entropy alloys, Laves phases, and Pd-containing alloys. Finally, an outlook is presented on current worldwide investments and future research directions for hydrogen-based energy storage.",

keywords = "catalysts, energy storage, hydrogen storage materials, intermetallic alloys, magnesium, multiscale modelling, nanostructure",

author = "Luca Pasquini and Kouji Sakaki and Etsuo Akiba and Allendorf, {Mark D.} and Ebert Alvares and Ares, {Jos{\`e} R.} and Dotan Babai and Marcello Baricco and {Bellosta Von Colbe}, Jos{\`e} and Matvey Bereznitsky and Buckley, {Craig E.} and Cho, {Young Whan} and Fermin Cuevas and {De Rango}, Patricia and Dematteis, {Erika Michela} and Denys, {Roman V.} and Martin Dornheim and Fern{\'a}ndez, {J. F.} and Arif Hariyadi and Hauback, {Bj{\o}rn C.} and Heo, {Tae Wook} and Michael Hirscher and Humphries, {Terry D.} and Jacques Huot and Isaac Jacob and Jensen, {Torben R.} and Paul Jerabek and Kang, {Shin Young} and Nathan Keilbart and Hyunjeong Kim and Michel Latroche and F. Leardini and Haiwen Li and Sanliang Ling and Lototskyy, {Mykhaylo V.} and Ryan Mullen and Orimo, {Shin Ichi} and Mark Paskevicius and Claudio Pistidda and Marek Polanski and Juli{\'a}n Puszkiel and Eugen Rabkin and Martin Sahlberg and Sabrina Sartori and Archa Santhosh and Toyoto Sato and Shneck, {Roni Z.} and S{\o}rby, {Magnus H.} and Yuanyuan Shang and Vitalie Stavila and Suh, {Jin Yoo} and Suwarno Suwarno and {Thi Thu}, Le and Wan, {Liwen F.} and Webb, {Colin J.} and Matthew Witman and Chubin Wan and Wood, {Brandon C.} and Yartys, {Volodymyr A.}",

note = "Publisher Copyright: {\textcopyright} 2022 The Author(s). Published by IOP Publishing Ltd.",

year = "2022",

month = jul,

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doi = "10.1088/2516-1083/ac7190",

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Pasquini, L, Sakaki, K, Akiba, E, Allendorf, MD, Alvares, E, Ares, JR, Babai, D, Baricco, M, Bellosta Von Colbe, J, Bereznitsky, M, Buckley, CE, Cho, YW, Cuevas, F, De Rango, P, Dematteis, EM, Denys, RV, Dornheim, M, Fernández, JF, Hariyadi, A, Hauback, BC, Heo, TW, Hirscher, M, Humphries, TD, Huot, J, Jacob, I, Jensen, TR, Jerabek, P, Kang, SY, Keilbart, N, Kim, H, Latroche, M, Leardini, F, Li, H, Ling, S, Lototskyy, MV, Mullen, R, Orimo, SI, Paskevicius, M, Pistidda, C, Polanski, M, Puszkiel, J, Rabkin, E, Sahlberg, M, Sartori, S, Santhosh, A, Sato, T, Shneck, RZ, Sørby, MH, Shang, Y, Stavila, V, Suh, JY, Suwarno, S, Thi Thu, L, Wan, LF, Webb, CJ, Witman, M, Wan, C, Wood, BC & Yartys, VA 2022, 'Magnesium- and intermetallic alloys-based hydrides for energy storage: Modelling, synthesis and properties', Progress in Energy, vol. 4, no. 3, 032007. https://doi.org/10.1088/2516-1083/ac7190

TY - JOUR

T1 - Magnesium- and intermetallic alloys-based hydrides for energy storage

T2 - Modelling, synthesis and properties

AU - Pasquini, Luca

AU - Sakaki, Kouji

AU - Akiba, Etsuo

AU - Allendorf, Mark D.

AU - Alvares, Ebert

AU - Ares, Josè R.

AU - Babai, Dotan

AU - Baricco, Marcello

AU - Bellosta Von Colbe, Josè

AU - Bereznitsky, Matvey

AU - Buckley, Craig E.

AU - Cho, Young Whan

AU - Cuevas, Fermin

AU - De Rango, Patricia

AU - Dematteis, Erika Michela

AU - Denys, Roman V.

AU - Dornheim, Martin

AU - Fernández, J. F.

AU - Hariyadi, Arif

AU - Hauback, Bjørn C.

AU - Heo, Tae Wook

AU - Hirscher, Michael

AU - Humphries, Terry D.

AU - Huot, Jacques

AU - Jacob, Isaac

AU - Jensen, Torben R.

AU - Jerabek, Paul

AU - Kang, Shin Young

AU - Keilbart, Nathan

AU - Kim, Hyunjeong

AU - Latroche, Michel

AU - Leardini, F.

AU - Li, Haiwen

AU - Ling, Sanliang

AU - Lototskyy, Mykhaylo V.

AU - Mullen, Ryan

AU - Orimo, Shin Ichi

AU - Paskevicius, Mark

AU - Pistidda, Claudio

AU - Polanski, Marek

AU - Puszkiel, Julián

AU - Rabkin, Eugen

AU - Sahlberg, Martin

AU - Sartori, Sabrina

AU - Santhosh, Archa

AU - Sato, Toyoto

AU - Shneck, Roni Z.

AU - Sørby, Magnus H.

AU - Shang, Yuanyuan

AU - Stavila, Vitalie

AU - Suh, Jin Yoo

AU - Suwarno, Suwarno

AU - Thi Thu, Le

AU - Wan, Liwen F.

AU - Webb, Colin J.

AU - Witman, Matthew

AU - Wan, Chubin

AU - Wood, Brandon C.

AU - Yartys, Volodymyr A.

PY - 2022/7/1

Y1 - 2022/7/1

N2 - Hydrides based on magnesium and intermetallic compounds provide a viable solution to the challenge of energy storage from renewable sources, thanks to their ability to absorb and desorb hydrogen in a reversible way with a proper tuning of pressure and temperature conditions. Therefore, they are expected to play an important role in the clean energy transition and in the deployment of hydrogen as an efficient energy vector. This review, by experts of Task 40 'Energy Storage and Conversion based on Hydrogen' of the Hydrogen Technology Collaboration Programme of the International Energy Agency, reports on the latest activities of the working group 'Magnesium- and Intermetallic alloys-based Hydrides for Energy Storage'. The following topics are covered by the review: multiscale modelling of hydrides and hydrogen sorption mechanisms; synthesis and processing techniques; catalysts for hydrogen sorption in Mg; Mg-based nanostructures and new compounds; hydrides based on intermetallic TiFe alloys, high entropy alloys, Laves phases, and Pd-containing alloys. Finally, an outlook is presented on current worldwide investments and future research directions for hydrogen-based energy storage.

AB - Hydrides based on magnesium and intermetallic compounds provide a viable solution to the challenge of energy storage from renewable sources, thanks to their ability to absorb and desorb hydrogen in a reversible way with a proper tuning of pressure and temperature conditions. Therefore, they are expected to play an important role in the clean energy transition and in the deployment of hydrogen as an efficient energy vector. This review, by experts of Task 40 'Energy Storage and Conversion based on Hydrogen' of the Hydrogen Technology Collaboration Programme of the International Energy Agency, reports on the latest activities of the working group 'Magnesium- and Intermetallic alloys-based Hydrides for Energy Storage'. The following topics are covered by the review: multiscale modelling of hydrides and hydrogen sorption mechanisms; synthesis and processing techniques; catalysts for hydrogen sorption in Mg; Mg-based nanostructures and new compounds; hydrides based on intermetallic TiFe alloys, high entropy alloys, Laves phases, and Pd-containing alloys. Finally, an outlook is presented on current worldwide investments and future research directions for hydrogen-based energy storage.

KW - catalysts

KW - energy storage

KW - hydrogen storage materials

KW - intermetallic alloys

KW - magnesium

KW - multiscale modelling

KW - nanostructure

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AN - SCOPUS:85137023724

SN - 2516-1083

VL - 4

JO - Progress in Energy

JF - Progress in Energy

IS - 3

M1 - 032007

ER -

Magnesium- and intermetallic alloys-based hydrides for energy storage: Modelling, synthesis and properties

Abstract

Bibliographical note

Keywords

UN SDGs

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