Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode

H. Singh; D. Donetsky; J. Liu; K. Attenkofer; B. Cheng; J. R. Trelewicz; I. Lubomirsky; E. Stavitski; A. I. Frenkel

doi:10.1063/1.5000679

Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode

H. Singh
, D. Donetsky
, J. Liu
, K. Attenkofer
, B. Cheng
, J. R. Trelewicz
, I. Lubomirsky
, E. Stavitski
, A. I. Frenkel

Stony Brook University
National Synchrotron Light Source II
Brookhaven National Laboratory
Institute for Advanced Computational Science
Weizmann Institute of Science

Research output: Contribution to journal › Article › peer-review

8 Scopus citations

Abstract

We report the development, testing, and demonstration of a setup for modulation excitation spectroscopy experiments at the Inner Shell Spectroscopy beamline of National Synchrotron Light Source - II. A computer algorithm and dedicated software were developed for asynchronous data processing and analysis. We demonstrate the reconstruction of X-ray absorption spectra for different time points within the modulation pulse using a model system. This setup and the software are intended for a broad range of functional materials which exhibit structural and/or electronic responses to the external stimulation, such as catalysts, energy and battery materials, and electromechanical devices.

Original language	English
Article number	045111
Journal	Review of Scientific Instruments
Volume	89
Issue number	4
DOIs	https://doi.org/10.1063/1.5000679
State	Published - 1 Apr 2018
Externally published	Yes

Bibliographical note

Publisher Copyright:
© 2018 Author(s).

Funding

The research leading to these results received funding through the NSF-BSF program. H.S. and A.I.F. acknowledge support by NSF Grant No. DMR-1701747. I.L. acknowledges the BSF Program Grant No. 2015679. J.R.T. acknowledges support from the NSF CAREER Program under Award No. CMMI-1554411. This research used 8-ID (ISS) beamline of the National Synchrotron Light Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Brookhaven National Laboratory under Contract No. DE-AC02-98CH10886. J.R.T. acknowledges the use of characterization resources in the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-SC0012704.

Funders	Funder number
DOE Office of Science
Office of Basic Energy Sciences
National Science Foundation
U.S. Department of Energy	DE-AC02-98CH10886, DE-SC0012704
Bloom's Syndrome Foundation	2015679
Office of Science
Brookhaven National Laboratory
Norsk Sykepleierforbund	DMR-1701747, CMMI-1554411
Institute for Functional Nanomaterials

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abstract = "We report the development, testing, and demonstration of a setup for modulation excitation spectroscopy experiments at the Inner Shell Spectroscopy beamline of National Synchrotron Light Source - II. A computer algorithm and dedicated software were developed for asynchronous data processing and analysis. We demonstrate the reconstruction of X-ray absorption spectra for different time points within the modulation pulse using a model system. This setup and the software are intended for a broad range of functional materials which exhibit structural and/or electronic responses to the external stimulation, such as catalysts, energy and battery materials, and electromechanical devices.",

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AU - Cheng, B.

AU - Trelewicz, J. R.

AU - Lubomirsky, I.

AU - Stavitski, E.

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Investigation of periodically driven systems by x-ray absorption spectroscopy using asynchronous data collection mode

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