Distribution of single-molecule line widths

E. Barkai; R. Silbey

doi:10.1016/s0009-2614(99)00797-6

Distribution of single-molecule line widths

E. Barkai, R. Silbey

Massachusetts Institute of Technology

Research output: Contribution to journal › Article › peer-review

28 Scopus citations

Abstract

Single molecule spectroscopy shows that line shapes of guest molecules in low-temperature disordered solids vary from one molecule to the other. We consider a single molecule in a host lattice interacting with randomly distributed two level defects via a long range interaction. We investigate in detail the dipolar interaction and calculate the probability density of variances for high and low densities of defects.

Original language	English
Pages (from-to)	287-295
Number of pages	9
Journal	Chemical Physics Letters
Volume	310
Issue number	3-4
DOIs	https://doi.org/10.1016/s0009-2614(99)00797-6
State	Published - 3 Sep 1999
Externally published	Yes

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10.1016/s0009-2614(99)00797-6

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title = "Distribution of single-molecule line widths",

abstract = "Single molecule spectroscopy shows that line shapes of guest molecules in low-temperature disordered solids vary from one molecule to the other. We consider a single molecule in a host lattice interacting with randomly distributed two level defects via a long range interaction. We investigate in detail the dipolar interaction and calculate the probability density of variances for high and low densities of defects.",

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AB - Single molecule spectroscopy shows that line shapes of guest molecules in low-temperature disordered solids vary from one molecule to the other. We consider a single molecule in a host lattice interacting with randomly distributed two level defects via a long range interaction. We investigate in detail the dipolar interaction and calculate the probability density of variances for high and low densities of defects.

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Distribution of single-molecule line widths

Abstract

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