Carbon Nanotube Reinforced Structural Composite Supercapacitor

Nitin Muralidharan, Eti Teblum, Andrew S. Westover, Deanna Schauben, Anat Itzhak, Merav Muallem, Gilbert D. Nessim, Cary L. Pint

Research output: Contribution to journalArticlepeer-review

60 Scopus citations

Abstract

Carbon nanotubes exhibit mechanical properties ideally suited for reinforced structural composites and surface area and conductivity attractive for electrochemical capacitors. Here we demonstrate the multifunctional synergy between these properties in a composite material exhibiting simultaneous mechanical and energy storage properties. This involves a reinforcing electrode developed using dense, aligned carbon nanotubes grown on stainless steel mesh that is layered in an ion conducting epoxy electrolyte matrix with Kevlar or fiberglass mats. The resulting energy storage composites exhibit elastic modulus over 5 GPa, mechanical strength greater than 85 MPa, and energy density up to 3 mWh/kg for the total combined system including electrodes, current collector, Kevlar or fiberglass, and electrolyte matrix. Furthermore, findings from in-situ mechano-electro-chemical tests indicate simultaneous mechanical and electrochemical functionality with invariant and stable supercapacitor performance maintained throughout the elastic regime.

Original languageEnglish
Article number17662
JournalScientific Reports
Volume8
Issue number1
DOIs
StatePublished - 5 Dec 2018

Bibliographical note

Publisher Copyright:
© 2018, The Author(s).

Funding

Funding for this work was provided by BSF Startup Grant Number - 2014041 and by a BSF Prof. Rahamimoff Travel Grant. G. D. N., E. T., A. I. and M. M. acknowledge partial support from the Israel Science Foundation and Israel Prime Minister’s Office fuel alternatives initiative under Israel Research Center for Electrochemical Propulsion (Grant: ISF 2797/11). We also acknowledge Dr. Leon Bellan and Dr. Lior Elbaz for some use of facilities and Keith Share, Adam Cohn, Landon Oakes, Rachel Carter, Anna Douglas and Jackson Meng for useful discussions and assistance in measurements.

FundersFunder number
BSF Prof. Rahamimoff
Bloom's Syndrome Foundation2014041
Israel Science FoundationISF 2797/11

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